Publisher's Synopsis
Excerpt from Electronic Structure and Bonding of Actinide Complexes
This report outlines some of the preliminary progress made in the study of the electronic structure of actinide complexes in the Hartree - Fock self - consistent - field approximation. Our goal is to interpret the optical and magnetic properties of these compounds and to estimate the degree to which covalency must be taken into account in order to understand the role of the 5f electrons in both molecular and metallic bonding. The specific compounds to be investigated will include both the hexafluoride and oxide complexes as well as small metallic clusters which reflect the complex geometry of the unit cell found in the metallic phase of these elements.
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